Economical test equipment is available for HF and VHF frequencies, but the ISM bands in this range are fairly narrow. More interesting are the higher ISM frequencies, e.g. the 900 MHz, 2.4 GHz, and 5 GHz bands. Unfortunately, commercial equipment for these frequencies is extremely expensive. However, the popularity of these bands for commercial applications has brought about the availability of a variety of high frequency integrated circuits at very low prices. These could be used to build instruments which, although not as accurate as expensive laboratory equipment, nevertheless provides useful functionality at a much lower price.
Also, there are no US ISM bands between 5 GHz and 24 GHz. 24 GHz is more of a challenge than we are equipped to take on. In fact 5 GHz is probably on the boundary of what we should attempt.
So, at least the 900 and 2.4 ISM bands should be supported. This should include the ability to measure harmonics, at least of 900 signals. Although power limitations for continuous operation in non-ISM bands are severe, allowed power for intermittent and periodic operation is significantly higher across most of the spectrum. Since the ISM bands are becoming increasingly crowded while many other parts of the spectrum are nearly empty, additional or full frequency coverage would support development of applications which could utilize this niche.